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CO2 methanation and co-methanation of CO and CO2 over Mn-promoted Ni/Al2

Kechao Zhao,Zhenhua Li,Li Bian

Frontiers of Chemical Science and Engineering 2016, Volume 10, Issue 2,   Pages 273-280 doi: 10.1007/s11705-016-1563-5

Abstract: A series of Mn-promoted 15 wt-% Ni/Al O catalysts were prepared by an incipient wetness impregnationThe effect of the Mn content on the activity of the Ni/Al O catalysts for CO methanation and the co-methanationThe presence of Mn increased the number of CO adsorption sites and inhibited Ni particle agglomerationThe Mn content was varied from 0.86% to 2.54% and the best CO conversion was achieved with the 1.71Mn-NiThe co-methanation tests on the 1.71Mn-Ni/Al O catalyst indicated that adding Mn markedly enhanced the

Keywords： Mn promotion     nickel catalysts     CO2 methanation     co-methanation of CO and CO2    

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Fe-Mn-sepiolite as an effective heterogeneous Fenton-like catalyst for the decolorization of reactive

Chengyuan SU,Weiguang LI,Xingzhe LIU,Xiaofei HUANG,Xiaodan YU

Frontiers of Environmental Science & Engineering 2016, Volume 10, Issue 1,   Pages 37-45 doi: 10.1007/s11783-014-0729-y

Abstract: A study of the decolorization of reactive brilliant blue in an aqueous solution using Fe-Mn-sepioliteMoreover, the Fe-Mn-sepiolite catalyst had good stability for the degradation of reactive brilliant blue

Keywords： Fe-Mn-sepiolite catalyst     heterogeneous Fenton-like     reactive brilliant blue     homogeneous precipitation    

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Denitrification performance and sulfur resistance mechanism of Sm–Mn catalyst for low temperature NH-SCR

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 5,   Pages 617-633 doi: 10.1007/s11705-022-2258-8

Abstract: MnOx and Sm–Mn catalysts were prepared with the coprecipitation method, and they showedsub>x by NH3 between 50 and 300 °C in the presence of excess oxygen. 0.10Sm–MnFor 0.10Sm–Mn catalyst, manganese sulfate and sulfur ammonium cannot be generated broadly under the influencesignificantly due to the addition of SO2, enhancing the sulfur resistance of the 0.10Sm–Mn

Keywords： MnOx     Sm–Mn     catalyst     NH3-SCR     sulfur resistance    

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Comparing the adsorption behaviors of Cd, Cu and Pb from water onto Fe-Mn binary oxide, MnO

Wei XU,Huachun LAN,Hongjie WANG,Hongming LIU,Jiuhui QU

Frontiers of Environmental Science & Engineering 2015, Volume 9, Issue 3,   Pages 385-393 doi: 10.1007/s11783-014-0648-y

Abstract: The adsorption potential of FMBO, FeOOH, MnO for the removal of Cd , Cu and Pb in aqueous systems was investigated in this study. Comparing to FMBO and FeOOH, MnO offered a much higher removal capacity towards the three metal ions. The maximal adsorption capacity of MnO for Cd , Cu and Pb were 1.23, 2.25 and 2.60 mmol·g , respectively. And that for FMBO were 0.37, 1.13, and 1.18 mmol·g and for FeOOH were 0.11, 0.86 and 0.48 mmol·g , respectively. The adsorption behaviors of the three metal ions on the three adsorbents were all significantly affected by pH values and heavy metal removal efficiency increased with pH increased. The Langmuir and Freundlich adsorption models were used to describe the adsorption equilibrium of the three metal ions onto the three adsorbents. Results showed that the adsorption equilibrium data fitted well to Langmuir isotherm and this indicated that adsorption of metal ions occurred on the three metal oxides adsorbents limited to the formation of a monolayer. More negative charged of MnO surface than that of FMBO and FeOOH could be ascribed by lower pH of MnO than that of FMBO and FeOOH and this could contribute to more binding sites on MnO surface than that of FMBO and FeOOH. The higher metal ions uptake by MnO than FMBO and FeOOH could be well explained by the surface charge mechanism.

Keywords： heavy metals     Fe-Mn binary oxide     manganese dioxide     ferric hydroxide     adsorption    

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Visible light induces bacteria to produce superoxide for manganese oxidation

Frontiers of Environmental Science & Engineering 2023, Volume 17, Issue 2, doi: 10.1007/s11783-023-1619-y

Abstract:

● Term of manganese-oxidizing microorganisms should be reconsidered.

Keywords： Mn(II) oxidation     Manganese-oxidizing bacteria     Reactive oxygen species     Mn(III/IV) oxides    

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Microwave-assisted catalytic oxidation of gaseous toluene with a Cu-Mn-Ce/cordierite honeycomb catalyst

Longli Bo, Shaoyuan Sun

Frontiers of Chemical Science and Engineering 2019, Volume 13, Issue 2,   Pages 385-392 doi: 10.1007/s11705-018-1738-3

Abstract: A novel Cu-Mn-Ce/cordierite honeycomb catalyst was prepared by an incipient wetness method and the catalystThe active ingredients were present as various spinel species of Cu, Mn and Ce oxides with differentAfter four consecutive cycles (a total of 1980 min), the Cu-Mn-Ce/cordierite catalyst still exhibited

Keywords： microwave     catalytic oxidation     toluene     Cu-Mn-Ce/cordierite     mineralization    

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Fluoride ions adsorption from water by CaCO enhanced Mn–Fe mixed metal oxides

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 2,   Pages 236-248 doi: 10.1007/s11705-022-2193-8

Abstract: Novel CaCO3-enhanced Mn–Fe mixed metal oxides (CMFC) were successfully prepared for the first

Keywords： mesoporous materials     metal oxides     fluoride ion     adsorption mechanism    

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Study on a green synthetic method of TRPPMCl (M= Fe, Mn, Co)

Jing FAN, Yuanbin SHE, Aixin WANG

Frontiers of Chemical Science and Engineering 2009, Volume 3, Issue 2,   Pages 222-223 doi: 10.1007/s11705-009-0059-y

Abstract: A series of TRPPMCl (M= Fe, Mn, Co) were synthesized through this innovative synthetic method, and these

Keywords： TRPPMCl metalloporphyrins     green synthesis     acid    

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Efficient promotion of methane hydrate formation and elimination of foam generation using fluorinated

Quan CAO, Dongyan XU, Huanfei XU, Shengjun LUO, Rongbo GUO

Frontiers in Energy 2020, Volume 14, Issue 3,   Pages 443-451 doi: 10.1007/s11708-020-0683-2

Abstract: Methane hydrate preparation is an effective method to store and transport methane. In promoters to facilitate methane hydrate formation, homogeneous surfactant solutions, sodium dodecyl sulfate (SDS) in particular, are more favorable than heterogeneous particles, thanks to their faster reaction rate, more storage capacity, and higher stability. Foaming, however, could not be avoided during hydrate dissociation with the presence of SDS. This paper investigated the ability of five fluorinated surfactants: potassium perfluorobutane sulfonate (PBS), potassium perfluorohexyl sulfonate (PHS), potassium perfluorooctane sulfonate (POS), ammonium perfluorooctane sulfonate (AOS), and tetraethylammonium perfluorooctyl sulfonate (TOS) to promote methane hydrate formation. It was found that both PBS and PHS achieve a storage capacity of 150 ( , the volume of methane that can be stored by one volume of water) within 30 min, more than that of SDS. Cationic ions and the carbon chain length were then discussed on their effects during the formation. It was concluded that PBS, PHS, and POS produced no foam during hydrate dissociation, making them promising promoters in large-scale application.

Keywords： methane hydrate     fluorinated surfactants     homogeneous promoter     foam elimination     stability    

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Effect of K and Ca on catalytic activity of Mn-CeO

Boxiong SHEN, Lidan DENG, Jianhong CHEN

Frontiers of Environmental Science & Engineering 2013, Volume 7, Issue 4,   Pages 512-517 doi: 10.1007/s11783-013-0519-y

Abstract: Mn-CeO /Ti-pillared clay (PILC) is an attractive catalyst for selective catalytic reduction of NO atThe poisoning of K and Ca on the catalyst of Mn-CeO /Ti-PILC is an important problem because K and CaX-ray photoelectron spectroscopy (XPS) were used to analyze the fresh and deactivated catalysts of Mn-CeO(Ca)Mn-CeO /Ti-PILC and (K)Mn-CeO /Ti-PILC are denoted for the dopes of the catalyst of Mn-CeO /Ti-PILCThe activities of Mn-CeO /Ti-PILC, (Ca)Mn-CeO /Ti-PILC and (K)Mn-CeO /Ti-PILC for NH -selective catalytic

Keywords： Mn-CeOx/Ti-pillared clay (PILC)     low-temperature selective catalytic reduction    

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NiBO (B = Mn or Co) catalysts for NH-SCR of NO at low-temperature in microwave field

Frontiers of Environmental Science & Engineering 2023, Volume 17, Issue 8, doi: 10.1007/s11783-023-1696-y

Abstract:

● Microwave-assisted catalytic NH3-SCR reaction over spinel oxides is carried out.

Keywords： Microwave field     Spinel oxides     NOx     Selective catalytic reduction    

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Amino acid promoted hydrogen battery system using Mn-pincer complex for reversible CO hydrogenation to

Frontiers in Energy 2022, Volume 16, Issue 5,   Pages 697-699 doi: 10.1007/s11708-022-0843-7

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Removal of elemental mercury with Mn/Mo/Ru/Al

Yongfu GUO, Naiqiang YAN, Ping LIU, Shijian YANG, Juan WANG, Zan QU

Frontiers of Environmental Science & Engineering 2013, Volume 7, Issue 3,   Pages 464-473 doi: 10.1007/s11783-012-0430-y

Abstract: In this work, a catalytic membrane using Mn/Mo/Ru/Al O as the catalyst was employed to remove elementalCompared with traditional catalytic oxidation (TCO) mode, Mn/Al O membrane catalytic system had muchof Mo and Ru, the production of Cl from the Deacon reaction and the retainability for oxidants over MnAs a result, the oxidization of Hg over Mn/Al O membrane was obviously promoted due to incorporationIn the presence of 8 ppmv HCl, the removal efficiency of Hg by Mn/Mo/Ru/Al O membrane reached 95% at

Keywords： flue gas     elemental mercury     membrane     catalysis     transition metal    

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Template-free synthesis of hierarchically macro-mesoporous Mn-TiO

Zhao Peng, Li-Hua Chen, Ming-Hui Sun, Pan Wu, Chang Cai, Zhao Deng, Yu Li, Wei-Hong Zheng, Bao-Lian Su

Frontiers of Chemical Science and Engineering 2018, Volume 12, Issue 1,   Pages 43-49 doi: 10.1007/s11705-017-1679-2

Abstract: This study described a template-free method for the synthesis of hierarchically macro-mesoporous Mn-TiOThe promoting effect of Mn doping and the hierarchically macro-mesoporous architecture on TiO basedThe results show that the catalytic performance of TiO based catalysts was improved greatly after MnMeanwhile, the Mn-TiO catalyst with the hierarchically macro-mesoporous architecture has a better catalytic

Keywords： titania     hierarchically macro-mesoporous structure     Mn-doping     selective catalytic reduction    

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Large-scale synthesis of isolated Mn2O3 nanotube/fiber with ferric nitrate as catalyst

ZHANG Aifei, LIU Jiping, L? Guangshu

Frontiers of Chemical Science and Engineering 2007, Volume 1, Issue 1,   Pages 55-58 doi: 10.1007/s11705-007-0011-y

Abstract: Isolated MnO nanotubes and nanofibers were prepared very easily at a large scale with the liquid-phase catalysis method. The MnO nanotubes had dimensions of 30 50 nm (exterior diameter) and 0.2 1.0 ?m (length), approximately. The O nanofibers had dimensions of 10 30 nm (diameter) and 0.4 2.0 ?m (length), approximately. Nano-O with different microstructures including nanotubes, nanofibers and nanoparticles could be selectively synthesized by controlling the contents and proportions of potassium permanganate and ferric nitrate. Ferric nitrate was an ideal catalyst for the preparation of O nanotube/fiber. When cobalt nitrate or nickel nitrate was used as catalyst, only amorphous nano-O was synthesized. X-ray diffraction (XRD) result shows that the O nanotube has a crystalline structure different from o-O, t-O, h-O and ?-O.

Keywords： different     nickel     exterior diameter     nanotube     XRD    

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Title Author Date Type Operation

CO2 methanation and co-methanation of CO and CO2 over Mn-promoted Ni/Al2

Kechao Zhao,Zhenhua Li,Li Bian

Journal Article

Fe-Mn-sepiolite as an effective heterogeneous Fenton-like catalyst for the decolorization of reactive

Chengyuan SU,Weiguang LI,Xingzhe LIU,Xiaofei HUANG,Xiaodan YU

Journal Article

Denitrification performance and sulfur resistance mechanism of Sm–Mn catalyst for low temperature NH-SCR

Journal Article

Comparing the adsorption behaviors of Cd, Cu and Pb from water onto Fe-Mn binary oxide, MnO

Wei XU,Huachun LAN,Hongjie WANG,Hongming LIU,Jiuhui QU

Journal Article

Visible light induces bacteria to produce superoxide for manganese oxidation

Journal Article

Microwave-assisted catalytic oxidation of gaseous toluene with a Cu-Mn-Ce/cordierite honeycomb catalyst

Longli Bo, Shaoyuan Sun

Journal Article

Fluoride ions adsorption from water by CaCO enhanced Mn–Fe mixed metal oxides

Journal Article

Study on a green synthetic method of TRPPMCl (M= Fe, Mn, Co)

Jing FAN, Yuanbin SHE, Aixin WANG

Journal Article

Efficient promotion of methane hydrate formation and elimination of foam generation using fluorinated

Quan CAO, Dongyan XU, Huanfei XU, Shengjun LUO, Rongbo GUO

Journal Article

Effect of K and Ca on catalytic activity of Mn-CeO

Boxiong SHEN, Lidan DENG, Jianhong CHEN

Journal Article

NiBO (B = Mn or Co) catalysts for NH-SCR of NO at low-temperature in microwave field

Journal Article

Amino acid promoted hydrogen battery system using Mn-pincer complex for reversible CO hydrogenation to

Journal Article

Removal of elemental mercury with Mn/Mo/Ru/Al

Yongfu GUO, Naiqiang YAN, Ping LIU, Shijian YANG, Juan WANG, Zan QU

Journal Article

Template-free synthesis of hierarchically macro-mesoporous Mn-TiO

Zhao Peng, Li-Hua Chen, Ming-Hui Sun, Pan Wu, Chang Cai, Zhao Deng, Yu Li, Wei-Hong Zheng, Bao-Lian Su

Journal Article

Large-scale synthesis of isolated Mn2O3 nanotube/fiber with ferric nitrate as catalyst

ZHANG Aifei, LIU Jiping, L? Guangshu

Journal Article